叶绿素荧光遥感在陆地生态系统碳循环和陆气相互作用中的应用研究进展          下载免费PDF全文

邱博  郭维栋 《大气科学学报》2022,45(6):801-814

陆地生态系统通过植被光合作用可以吸收约30％的人为碳排放,在全球碳循环、减缓大气二氧化碳浓度上升等方面具有重要作用。最近10年发展起来的日光诱导叶绿素荧光遥感技术,可以监测植被实际光合作用,为全球陆地生态系统碳循环的研究提供了新的思路和方法。本文回顾了叶绿素荧光遥感产品发展及其在陆地生态系统碳循环和陆气相互作用中的应用研究进展,特别是在全球植被总初级生产力估算和陆地生态系统碳循环模型发展方面的进展,并进一步讨论了该领域研究面临的挑战和未来的发展方向。  相似文献   

青藏高原高寒草地小流域水体碳氮输出特征及其影响因素          下载免费PDF全文

杜陈军  张梦瑶  高永恒 《水文》2018,38(2):46-52

以青藏高原长江源区典型高寒草地小流域为研究对象,基于2012年小流域气象监测数据和小流域径流水样分析,探讨了小流域水体碳氮输出特征,分析了气象因子和土壤水热对小流域水体碳氮输出的影响。结果表明,径流水体碳氮质量浓度均较低,其中可溶性有机碳(DOC)、可溶性有机氮(DON)、铵态氮(NH4+-N)和硝态氮(NO3--N)含量分别在2.95~6.96mg.L-1、0.45~1.15mg.L-1、0.02~0.88mg.L-1和0.16~0.36mg.L-1之间;DOC、DON、NO3--N在8~10月份之间随时间逐渐升高,9月中旬达到峰值后波动下降,NH4+-N无显著的季节变化特征,溶解氮中DONNO3--NNH4+-N;DOC和DON的输出量与降水、不同土层(20、40、60、90、120cm)地温和不同深度(10、20、40、60cm)土壤水分、水温呈极显著正相关(P0.001),与90、120cm土壤水分呈极显著负相关(P0.001);NH4+-N的输出量与降水、气温、水温呈显著正相关(P0.05);NO3--N与降水呈极显著正相关(P0.001)。  相似文献   

俯冲带碳酸盐化对深部碳循环的启示:以中国西南天山碳酸盐化云母片岩为例   总被引：1，自引：1，他引：0  

彭卫刚  张立飞  申婷婷  胡晗 《岩石学报》2018,34(4):1204-1218

俯冲带可将地球表层碳输送至深部地幔,同时也记录着俯冲板片来源碳质流体的迁移沉淀机制,对地球深部碳循环具有重大影响。近年来,俯冲带脱碳机制的研究表明流体溶解脱碳作用是冷的大洋俯冲板片释放COH流体的重要方式,而上覆板块(尤其地幔楔)则被认为是缓冲这些COH流体的重要场所,甚至是俯冲带CO_2的唯一"归宿"。事实上,俯冲带岩石本身的固碳能力却受到了忽视,而对俯冲带岩石捕获和固存CO_2(carbon capture and storage,CCS)能力的评估对全球碳通量的估算尤为重要。本文以中国西南天山高压-超高压变质带中碳酸盐化云母片岩为例,探讨俯冲带岩石的碳酸盐化对深部碳循环的影响。西南天山长阿吾子一带的碳酸盐化云母片岩记录了俯冲板片起源的碳质流体对俯冲带云母片岩的交代作用,地球化学特征表明蛇纹岩释放的富水流体溶解俯冲洋壳中的碳酸盐可能是产生COH流体的重要机制。基于碳质流体对多硅白云母(Si(a.p.f.u.)=3.58～3.73)的交代及相对高压的碳酸盐矿物(主要为白云石和菱镁矿)与金红石的共生,结合区域上碳酸盐化云母片岩与高压碳酸盐化蛇纹岩(HP-ophidolomite)的伴生,我们认为云母片岩的碳酸盐化作用可能发生在俯冲板片峰期稍后的高压折返阶段。俯冲带云母片岩的固碳作用表明除了上覆板块,俯冲带岩石本身对于碳质流体也具有很好的吸收能力。初步估算表明俯冲带云母片岩的碳酸盐化每年可固存至少2.46～6.68Mt/yr,约占俯冲板片每年进碳量的4%～17%。  相似文献   

Comparative Study of Hydrogen and Carbon Isotopic Composition of Gases Generated from the Pyrolysis of a Peat under Saltwater and Freshwater Conditions     

WU Yingzhong  DUAN Yi  ZHAO Yang  CAO Xixi  MA Lanhu  QIAN Yaorong  LI Zhongping  XING Lantian 《《地质学报》英文版》2018,92(5):1879-1887

To understand the influence of the diagenetic water medium on the isotopic compositions of thermogenic coalbed gas, both hydrous and anhydrous closed-system pyrolyses were performed at temperatures of 250°C to 650°C on an herbaceous marsh peat. Compared to the results of anhydrous pyrolysis, the hydrocarbon gases generated from hydrous pyrolyses have very different hydrogen isotopic compositions. However, the carbon isotopic compositions of the hydrocarbon gases became only slightly heavier in hydrous pyrolysis, compared to that from anhydrous pyrolysis. With the progress of thermal evolution from peat to a more advanced thermal maturity of vitrinite reflectance values (Ro) of 5.5% during the pyrolysis, the difference in the average δD value increased from 52‰ to 64‰ between the hydrous pyrolysis with saltwater and anhydrous pyrolysis and increased from 18‰ to 29‰ between the hydrous pyrolysis with freshwater and anhydrous pyrolysis, respectively. The difference in the average δ13C value was only 1‰–2‰ between the hydrous and anhydrous pyrolysis. The relationships between the δD values of the generated hydrocarbon gases and Ro values as well as among δD values of the hydrocarbon gas species are established. The close relationships among these parameters suggest that the water medium had a significant effect on the hydrogen isotopic composition and a minimal effect on the carbon isotopic composition of the hydrocarbon gases. The results of these pyrolyses may provide information for the understanding of the genesis of coalbed gas from herbaceous marsh material with the participation of different diagenetic water media.  相似文献   

元素分析仪-同位素比值质谱测量碳氮同位素比值最佳反应温度和进样量的确定   总被引：2，自引：2，他引：0  

徐丽  邢蓝田  王鑫  李中平  毛俊丽 《岩矿测试》2018,37(1):15-20

沉积有机质的碳氮稳定同位素值是进行古气候、古环境及生态系统研究不可或缺的主要研究手段,目前碳氮同位素主要利用元素分析仪-同位素比值质谱(EA-IRMS)系统来测定。EA-IRMS测定过程中的反应温度及样品进样量直接影响反应物在测试中的燃烧程度,从而影响测试数据的精度。本文利用EA-IRMS技术,以标准样品为参考,在不同转化温度下测试碳氮同位素值,研究保证测试精度的最佳反应温度条件;同时,通过分析不同含氮量样品的检测限,明确了样品含氮量与最低检测限之间的关系,确定了精确测定氮同位素值的最低进样量。结果表明:反应温度对测试精度有显著影响,在碳同位素测定时,将反应温度设定为900℃或以上时测试精度均能达到±0.2‰;氮同位素测定时,反应温度须设定为950℃时测试精度才能达到±0.3‰。实验得出样品含氮量与检测限之间的线性相关性为R2=0.873,开展氮同位素测定时可根据此关系来判断和控制进样量。  相似文献   

全球LNG海上运输网络演化及中国贸易现状分析     

梅强  胡勤友  刘希亮  赵瑞娜  杨春  王鹏  戚玉玲  杨洋  袁启睿 《地球信息科学学报》2022,24(9):1701-1716

随着“碳达峰”、“碳中和”发展目标的提出,液化天然气（Liquefied Natural Gas,简称LNG）作为清洁低碳能源逐渐受到能源市场的重视。在此背景下,重点分析LNG海上运输网络演化模式,对掌握全球能源格局动态和中国的进口贸易现状具有重要意义。本文利用船舶轨迹数据和复杂网络理论,聚焦2018—2020年全球LNG海上运输网络演化趋势;同时针对中国的贸易现状,重点分析中国LNG进口来源、主要进口港分布及进口量排名前三的进口港的货源流入状况。结果表明：① 2018—2020年,全球LNG海上运输网络呈扩大趋势,并呈现出“无标度”特性;同时骨干网络节点连接的“广度”和“深度”正在增强,全球LNG贸易存在趋于垄断的风险;② “一带一路”国家贸易参与度强,中北美、南亚和东南亚地区的进口港数量和进口航次数增长尤为明显,萨贝塔、邦尼按照贸易出口量排名已进入全球前八;③ 网络的平均最短路径值在2018—2020年逐年递增,“转运港”业务新模态逐渐兴起;截止到2020年共有21个转运港口参与LNG贸易中,美国占据全球转运的主导地位;④ 中国的LNG进口货量规模发展迅速,海上运输网络流向趋于多元,但澳大利亚仍占据主要来源地位;按照进口量统计天津港、深圳港和永安港排名前三,“减碳”压力促使经济发达地区建设接收站并且不断增大进口量。  相似文献   

Characteristics of Lake Breezes and Their Impacts on Energy and Carbon Fluxes in Mountainous Areas     

Lujun XU  Huizhi LIU  Qun DU  Yang LIU  Jihua SUN  Anlun XU  Xiaoni MENG 《大气科学进展》2021,38(4):603-614

In mountainous lake areas, lake–land and mountain–valley breezes interact with each other, leading to an "extended lake breeze". These extended lake breezes can regulate and control energy and carbon cycles at different scales. Based on meteorological and turbulent fluxes data from an eddy covariance observation site at Erhai Lake in the Dali Basin,southwest China, characteristics of daytime and nighttime extended lake breezes and their impacts on energy and carbon dioxide exchange in 2015 are investigated. Lake breezes dominate during the daytime while, due to different prevailing circulations at night, there are two types of nighttime breezes. The mountain breeze from the Cangshan Mountain range leads to N1 type nighttime breeze events. When a cyclonic circulation forms and maintains in the southern part of Erhai Lake at night, its northern branch contributes to the formation of N2 type nighttime breeze events. The prevailing wind directions for daytime, N1, and N2 breeze events are southeast, west, and southeast, respectively. Daytime breeze events are more intense than N1 events and weaker than N2 events. During daytime breeze events, the lake breeze decreases the sensible heat flux(Hs) and carbon dioxide flux(F_{CO_2}) and increases the latent heat flux(LE). During N1 breeze events, the mountain breeze decreases Hs and LE and increases F_{CO_2}. For N2 breeze events, the southeast wind from the lake surface increases Hs and LE and decreases suppress carbon dioxide exchange.  相似文献   

The First Global Carbon Dioxide Flux Map Derived from TanSat Measurements     

Dongxu YANG  Yi LIU  Liang FENG  Jing WANG  Lu YAO  Zhaonan CAI  Sihong ZHU  Naimeng LU  Daren LYU 《大气科学进展》2021,38(9):1433-1443

Space-borne measurements of atmospheric greenhouse gas concentrations provide global observation constraints for top-down estimates of surface carbon flux.Here,the first estimates of the global distribution of carbon surface fluxes inferred from dry-air CO_2 column (XCO_2) measurements by the Chinese Global Carbon Dioxide Monitoring Scientific Experimental Satellite (Tan Sat) are presented.An ensemble transform Kalman filter (ETKF) data assimilation system coupled with the GEOS-Chem global chemistry transport model is used to optimally fit model simulations with the Tan Sat XCO_2 observations,which were retrieved using the Institute of Atmospheric Physics Carbon dioxide retrieval Algorithm for Satellite remote sensing (IAPCAS).High posterior error reduction (30%–50%) compared with a priori fluxes indicates that assimilating satellite XCO_2 measurements provides highly effective constraints on global carbon flux estimation.Their impacts are also highlighted by significant spatiotemporal shifts in flux patterns over regions critical to the global carbon budget,such as tropical South America and China.An integrated global land carbon net flux of 6.71±0.76 Gt C yr~(-1) over12 months (May 2017–April 2018) is estimated from the Tan Sat XCO_2 data,which is generally consistent with other inversions based on satellite data,such as the JAXA GOSAT and NASA OCO-2 XCO_2 retrievals.However,discrepancies were found in some regional flux estimates,particularly over the Southern Hemisphere,where there may still be uncorrected bias between satellite measurements due to the lack of independent reference observations.The results of this study provide the groundwork for further studies using current or future Tan Sat XCO_2 data together with other surfacebased and space-borne measurements to quantify biosphere–atmosphere carbon exchange.  相似文献   

Seeking a handle on climate change: Examining the comparative effectiveness of energy efficiency improvement and renewable energy production in the United States     

《Global Environmental Change》2021

This study examines the comparative effectiveness of two important proposed solutions to climate change—energy efficiency improvement and the development and use of renewable energy sources. We focus specifically on their impacts on carbon dioxide emissions by conducting fixed effects regression analysis of panel data pertaining to U.S. states. The analysis reveals a negative relationship between both remedies and carbon dioxide emissions. Although the effects of these potential solutions are statistically equivalent, renewable energy production has a slight edge. Reflecting upon these findings and the larger environmental problem, we caution against exclusive reliance on efficiency improvement and renewable energy to the neglect of other important actions, such as lifestyle modifications. A broad range of social changes, which incorporate the remedies investigated in this paper, are needed to limit long-term global temperature increases to the desired level.  相似文献   

大气气溶胶中的铁及其溶解度研究综述          下载免费PDF全文

齐宇轩  周杨 《山东气象》2021,41(2):1-13

生物活性铁(Fe) 进入生物地球化学循环中能够调节碳循环,影响海洋初级生产力,间接影响全球气候变化。决定 Fe生物可利用度的关键因子是可溶Fe含量,其中大气气溶胶的长距离传输是上层海洋获取生物可利用Fe的重要来源。近年来,对气溶胶中的Fe及溶解度的研究取得了重要进展,包括对不同区域Fe质量浓度和溶解度的观测以及对Fe溶解度影响因素的讨论。基于以上研究成果,汇总了近二十年全球部分陆地和海洋站点观测所得的不同粒径气溶胶颗粒物中的Fe质量浓度及其溶解度数据;重点介绍了气溶胶沉降入海洋前影响Fe溶解度的主要因素,包括Fe的来源、大气物理过程以及大气化学和传输混合过程等,并就各影响因素间的关联及相对重要性展开讨论;对未来气溶胶 Fe的研究方向和方法提出建议。  相似文献